Let me start by complimenting you on a very clear description plus illustration of the balancing act. But you should not have drilled those
holes where you did. As a rule of thumb, a good press fit requires that a big end pin hole should be surrounded by at least half its diameter in material. So for a 20 mm pin there should be at least 10 mm of crank web material everywhere around the hole. As you can see, the large original balancing
holes already intrude into this zone, and with the small
holes you added there will be little stiffness left.

Removing material in the blue circles would have been a safer approach, although it might not haved raised the balance factor sufficiently.
The best way would be to remove material from the inside faces of the crank webs, around the big end recesses. That would have two additional benefits: it would improve lubrication and cooling of the big end bearing and it would enlarge the crankcase volume.
Now that I am grumbling anyway: big end pins should be massive. The large void in the pictured pin is not exactly promoting a good press fit.
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